Interlayer pairing mechanism for bilayer nickelate superconductors
cond-mat.supr-con, cond-mat.str-el
Submitted: 2026-06-13
Updated: 2026-09-17
Comments: 36 pages, 8 figures, 2 tables
License: http://creativecommons.org/licenses/by/4.0/
The gist: The discovery of superconductivity in Ruddlesden-Popper bilayer nickelates under both high pressure and ambient conditions has opened a new paradigm for exploring unconventional superconductivity.
Terminology
Abstract
The discovery of superconductivity in Ruddlesden-Popper bilayer nickelates under both high pressure and ambient conditions has opened a new paradigm for exploring unconventional superconductivity. This review provides a brief survey of theoretical progress on bilayer nickelate superconductors. Drawing from the key experimental observations, we summarize essential physical ingredients including the hybridized Ni-3 d x 2-y squared and 3 d z squared electronic structure, orbital-dependent electronic correlation, Hund's coupling, and strong interlayer magnetic coupling. The fundamental theoretical models including the bilayer two-orbital Hubbard model and its minimal t - J variants are introduced. Starting from the atomic-limit interlayer valence bond picture of the half-filled d z squared orbital, we elaborate on strong correlation interlayer pairing mechanisms based on different limiting considerations. Specific emphasis is placed on the hybridization mechanism, where the d z squared local singlet pairs provide the pairing energy and their hybridization with itinerant d x 2-y squared promotes superconducting phase coherence. We further analyze the pairing symmetry, the dependence of T c on various internal and external parameters, the nontrivial normal state properties including the Fermi liquid, non-Fermi liquid, weakly insulating and pseudogap behaviors. Effects of pressure tuning, oxygen content, and Kondo scattering induced by oxygen vacancies are also discussed. Finally, weak correlation theories based on spin fluctuations associated with Fermi surface nesting are briefly covered.
Sources
- High-temperature superconductivity in Nd$_{0.85}$Sr$_{0.15}$NiO$_2$ membranes under pressure
- Enhanced and robust superconductivity in La0.8Sr0.2NiO2 membranes compressed up to 210 GPa
- Nature of magnetism in bilayer nickelate La3Ni2O7 single crystals
- Interlayer electronic coherence links magnetism and superconductivity in Ruddlesden-Popper nickelates
- Regulating oxygen content and superconductivity in La 3 Ni 2 O 7+ delta
- Direct Observation of d-Wave Superconducting Gap Symmetry in Pressurized La3Ni2O7-delta Single Crystals
- Electronic structure of compressively strained thin film La$_2$PrNi$_2$O$_7$
- Electronic structures across superconductor-insulator transition in Ruddlesden-Popper bilayer nickelate films
- Observation of superconductivity-induced leading-edge gap in Sr-doped $\mathrm{La}_{3}\mathrm{Ni}_{2}\mathrm{O}_{7}$ thin films
- A superconducting half-dome in bilayer nickelates
- $3d_{z^2}$ orbital delocalization and magnetic collapse in superconducting (La,Pr)$_3$Ni$_2$O$_{7-\delta}$ films
- Doping evolution of spin excitations in La$_{3-x}$Sr$_{x}$Ni$_2$O$_7$/SrLaAlO$_4$ superconducting thin films
- Atomically resolved intrinsic superconducting gap in (La,Pr)3Ni2O7 films
- Interlayer Five-Spin Polaron in Superconducting Bilayer Nickelates
- Pressure-induced superconductivity in epitaxially-stabilized Pr$_3$Ni$_2$O$_7$ films
- Electron-like high-temperature superconductivity induced by compressive strain in La2PrNi2O7 thin films
- Thermodynamic phase transition, pairing symmetry and Fermi surface topology in Ruddlesden-Popper nickelate films
- Structural and Electronic Evolution of Bilayer Nickelates Under Biaxial Strain
- Theoretical study on the electronic properties and multiorbital models of La$_3$Ni$_2$O$_7$ thin films on SrLaAlO$_4$ (001)
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