EPR as a probe for the mechanisms of chirality-induced spin selectivity in photoinduced charge transfer
The study investigates radical pair states in photoinduced charge transfer to understand chirality-induced spin selectivity (CISS). By computing electron-paramagnetic resonance spectra, the research identifies peculiar signatures of different spin states. This helps determine which microscopic models—like those involving Dzyaloshinskii-Moriya interactions—are experimentally accessible and how to verify them.